Robust control design for quantum systems is a challenging and key task for practical technology. In this work, we apply neural networks to learn the control problem for the semiclassical Schr\"odinger equation, where the control variable is the potential given by an external field that may contain uncertainties. Inspired by a relevant work [29], we incorporate the sampling-based learning process into the training of networks, while combining with the fast time-splitting spectral method for the Schr\"odinger equation in the semiclassical regime. The numerical results have shown the efficiency and accuracy of our proposed deep learning approach.
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