Transition metal dichalcogenides have recently emerged as promising two-dimensional materials with intriguing electronic properties. Existing calculations of intrinsic phonon-limited electronic transport so far have concentrated on the semicondcucting members of this family. In this paper we extend these studies by investigating the influence of electron-phonon coupling on the electronic transport properties and band renormalization of prototype inherent metallic bulk and monolayer TaS$_2$. Based on density functional perturbation theory and semi-classical Boltzmann transport calculations, promising room temperature mobilities and sheet conductances are found, which can compete with other established 2D materials, leaving TaS$_2$ as promising material candidate for transparent conductors or as atomically thin interconnects. Throughout the paper, the electronic and transport properties of TaS$_2$ are compared to those of its isoelectronic counterpart TaSe$_2$ and additional informations to the latter are given. We furthermore comment on the conventional su- perconductivity in TaS$_2$, where no phonon-mediated enhancement of TC in the monolayer compared to the bulk state was found.
翻译:在本文件中,我们扩大了这些研究的范围,调查电子-光电联动对电子运输特性的影响,以及原金属内散体和单层TAS$2的带状重新整顿原型金属和单层TAS$2美元。根据密度功能扰动理论和半古典博尔茨曼运输计算、有希望的房间温度波动和床单导导体,可以与其他固定的2D材料竞争,使TAS$2成为有希望的材料候选透明导体或原子薄线连接。在本文中,TAS$2的电子和运输属性与其偏电子对应TASe$2美元相比,与后者相比,还提供了其他信息。我们进一步评论了TAS$2的常规透视率,因为发现在这种状态下,单层的三角合作在单层与状态之间没有发生非震荡式的增强。